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After recording further songs for Immediate Records, which remain unreleased, and making a brief appearance in the 1967 documentary Tonite Let's All Make Love in London, performing her song "Winter Is Blue", she decided to travel with her boyfriend Robert Lewis by horse and cart to the Hebridean Islands to join a commune planned by a friend, fellow folk singer Donovan ("from South London up to the Hebrides. Initially to Skye but we carried on to the Outer Hebrides."). During the trip she began writing the songs that eventually became her first album, Just Another Diamond Day.
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In 2000, Just Another Diamond Day was re-released on CD (with bonus tracks), assuring her influence over a new generation of folk artists such as Devendra Banhart and Joanna Newsom. In 2001, Banhart wrote to her asking for her advice, beginning her connection with many of the contemporary performers who cite her work. In 2002, she was invited by Piano Magic musician Glen Johnson to sing guest vocals on his song "Crown of the Lost", her first recording in over 30 years. Since then, she has appeared on releases by Devendra Banhart and Animal Collective and, in 2005, she recorded and released her second album, Lookaftering on Fat Cat Records, some 35 years after her first. The album was produced by composer Max Richter and featured many of her contemporary followers including Banhart, Joanna Newsom, Adem, Kevin Barker of Currituck Co, Otto Hauser of Espers and Adam Pierce of Mice Parade. It was well received by critics and fans alike.
During the autumn of 2006, Bunyan assembled an ad hoc band and embarked on a brief North American tour, with performances in both Canada and the US. She performed songs from both of her solo albums, as well as some of the rare material from the unreleased Oldham sessions.
Her music reached a much wider audience when "Just Another Diamond Day" was used in a TV advert for a mobile phone company.
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October 2007 saw the release of a compilation album of her mid-1960s singles and unreleased demos recorded at the time entitled Some Things Just Stick in Your Mind - Singles and Demos 1964 to 1967.
2007 also saw Vashti provide vocals on three songs for former Jack frontman Anthony Reynolds' debut solo album British Ballads. Bunyan sang with Reynolds on the songs "Country Girl", "Just So You Know" and "Song Of Leaving".
In January 2008, Vashti said she was recording a new album. "I’m supposed to be writing just now. I have one complete song and a whole lot of fragments. I’m supposed to have them finished by May and there’s no way. I’m hoping, and the plan is, I’ll be working with Andy Cabic of Vetiver."
In June 2008, Vashti appeared at London's Royal Festival Hall with The Heritage Orchestra as part of Massive Attack's Meltdown, in a live performance of Vangelis' Blade Runner soundtrack, singing "Rachael's Song" as sung by Mary Hopkin on the original recorded soundtrack.
On 25 October 2008, Vashti Bunyan: From Here To Before, a feature documentary directed by Kieran Evans had its world premieres at the Times BFI London Film Festival. The film retraces Bunyan’s journey across the British Isles and sets it against the backdrop of her first high-profile London concert. It uses her trip through Britain as its main narrative structure, accompanying her as she retraces her extraordinary journey. The album provides the soundtrack to that journey, just as it did the first time.
Bunyan's cover of the late John Martyn's "Head and Heart" will appear on an upcoming tribute album, titled "Johnny Boy Would Love This. A Tribute to John Martyn."
Discography
Studio albums
Just Another Diamond Day (Philips 1970)
Lookaftering (Fat Cat Records 2005)
Compilations
Some Things Just Stick in Your Mind – Singles and Demos 1964 to 1967 (Fat Cat Records/Spinney Records 2007)
Singles
"Some Things Just Stick in Your Mind" / "I Want To Be Alone" (Decca, 1965) (as Vashti)
"Train Song" / "Love Song" (Columbia (EMI), 1966) (as Vashti)